NPU, or nice part usage, means using a LEGO element for something other than what it was designed to be. A frog becomes a blossom, a minifigure tool becomes a valve, a piece of armour becomes a petal. The part is chosen for its shape, colour and way of connecting, not its name. LEGO's own designers do it in official sets, which makes those sets the best place to start learning.
Quick answer: study how official sets repurpose parts, then practise looking at every element for its shape and connection points instead of what it is called.
Documented examples from official sets
The Botanicals line is the best-known showcase of NPU in LEGO's own designs, and reviewers have documented the choices in detail.
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Bonsai Tree (10281). The cherry blossom version of the tree uses 100 pink frogs among the branches as blossoms, as New Elementary's review describes. The frog is Animal, Frog (33320).
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Orchid (10311). According to The Brothers Brick, a frog forms the centre of each flower, a printed Demogorgon head from Stranger Things forms the hood on the buds, and large-figure shoulder armour turns up among the parts. The review notes the set uses new colours of existing parts rather than new moulds.
Bonsai Tree
$49.99
Bonsai Tree: green foliage or a cherry blossom crown, the blossoms made with pink frogs.
Orchid
$49.99
Orchid: flower centres made from frogs and bud hoods from a Demogorgon head, all from existing parts.
How to train your eye
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Look at shape, not name. Ignore what a part is called. A curved armour piece is a petal, a roof or a hull panel; a round tile is a button, a light or a bolt.
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Check how it connects. A great shape is only useful if it attaches. Look for studs, anti-studs, clips, bars and pin holes on every unusual part.
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Study official instructions. LEGO publishes building instructions free on LEGO.com. Paging through a Botanicals, Architecture or modular set shows where designers used a part in an unexpected place.
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Follow parts-focused writing. Sites such as New Elementary review sets with a focus on the parts and how they are used.
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Keep a test tray. Keep a handful of odd parts on your desk and try them in places they do not belong. Photograph combinations that work.
Parts that repurpose well
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Animal figures and minifigure accessories: frogs, tools, food and headgear have distinctive shapes and a way to attach.
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Plant elements: leaves and stems work as feathers, flames, water or texture.
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Clips, bars and handles: plates such as 61252 and 26047 let you attach parts at angles.
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Round plates and tiles: 6141 and 98138 become lights, buttons, rivets and flower centres.
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Small Technic parts: pins, bushes and small gears suggest machinery when left exposed.
Where NPU meets other techniques
NPU often goes together with greebling, where repurposed parts become surface detail, and with SNOT building, which lets you attach a part sideways or upside down so its best side faces out. When you are missing a part entirely, see our guide to LEGO part substitutes.